Magnetic order and enhanced exchange in the quasi-one-dimensional molecule-based antiferromagnet Cu(NO3)2(pyz)3 [dataset]

Tom Lancaster, Benjamin M Huddart, Jamie Brambleby, Paul A Goddard, Fan Xiao, Stephen J Blundell, Francis L Pratt, John Singleton, Piero Macchi, Rebecca Scatena, Alyssa M Barton & Jamie L Manson
The quasi-one-dimensional molecule-based Heisenberg antiferromagnet Cu(NO3)2(pyz)3 has an intrachain coupling J = 13.7(1) K and exhibits a state of long-range magnetic order below TN = 0.105(1) K. The ratio of interchain to intrachain coupling is estimated to be |J′/J| = 3.3 × 10−3, demonstrating a high degree of isolation for the Cu chains.
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