Electronic spin states in fullerides and endohedral fullerenes

Jürgen Rahmer
This PhD thesis presents a study of electronic properties and spin states of fullerene materials using high-field electron-spin resonance (ESR) operating at frequencies of 95 GHz (W band) and standard-field ESR operating at 9 GHz (X band). Investigated carbon-cage materials range from solid fullerene salts like alkali fullerides (1), bis(arene)chromium fullerides (2), and mixed alkali/alkaline-earth fullerides (3), over fullerenium salts (4) to molecular systems like the metallofullerene Sc3@C82 (5). 1) Investigations of the alkali fullerides...
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