Synthesis, structure and electrical properties of the two-dimensional organic conductor, (BEDT-TTF)2BrI2

Daoben Zhu, Ping Wang, Meixiang Wan, Zhaolou Yu, Nailue Zhu, Stephan Gärtner & Dieter Schweitzer
Single crystals of α-(BEDT-TTF)2BrI2 and β-(BEDT-TTF)2BrI2 were prepared using standard electrochemical techniques in nitrogen saturated benzonitrile using containing (n-C4H10)NBrI2 as supporting electrolyte. The crystals have nearly identical structure features of α-(BEDT-TTF)2I3 and β-(BEDT-TTF)2I3, except that the BrI−2 anions are disordered in α-(BEDT-TTF)2BrI2 and β-(BEDT-TTF)2BrI2. Their electrical behavior is different from the corresponding α-,β-(BEDT-TTF)2I3 species.
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