Motivated by the cluster structure of two-loop scattering amplitudes in N = 4 Yang-Mills theory we define cluster polylogarithm functions. We find that all such functions of weight 4 are made up of a single simple building block associated to the A2 cluster algebra. Adding the requirement of locality on generalized Stasheff polytopes, we find that these A2 building blocks arrange themselves to form a unique function associated to the A3 cluster algebra. ThisA3 function...