Data for spin quantum beats in pump push spectroscopy

Christoph Lambert, David Mims, Jonathan Herpich, Nikita Lukzen & Ulrich Steiner
Spin quantum beats prove the quantum nature of reactions involving radical pairs, the key species of spin chemistry. However, such quantum beats remain hidden to transient-absorption-based optical observation because the spin hardly affects the radical pairs’ absorption properties. We succeeded in demonstrating such quantum beats in the photo-induced charge separated state (CSS) of an electron-donor-acceptor dyad by using two laser pulses, one for pumping the sample, and another one, with variable delay, for further exciting...
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