Ultrafast dynamics from quantum to classical regime

Hui Li
This thesis presents work on the interaction of waveform controlled few-cycle pulses with various systems, from simple diatomic molecules through hydrocarbons and C60 fullerene, to nano-sized silver clusters. By employing the single-shot phase-tagged velocity-map imaging (VMI) technique, the angular distributions of ionic fragmentations and electrons can be obtained. Various electronic and molecular dynamics can be manipulated by controlling, e.g. carrier envelope phase (CEP), laser intensity, and polarization of few-cycle pulses. The dissociative ionization in the...
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