Linking the solid state and solution thorium aqua structures: A solid state powder neutron diffraction investigation

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A understanding of the aqueous chemistry of the actinide ions is not as well developed as for transition metals or the lanthanides. Fundamentally important information such as the number of coordinated water molecules is still under debate. This has relied on EXAFS, but this technique cannot give precise coordination numbers. In this work we aim, for the first time, to use neutron diffraction techniques to explicitly locate the coordinated water molecules in three thorium compounds...
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