Inelastic neutron scattering studies on novel frustrated antiferromagnets Li3Mg2MO6 (M = Ru, Os)

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A newly discovered novel frustrated antiferromagnets Li3Mg2MO6 (M = Ru, Os) constitutes edge-sharing triangles of M4+ ions (S = 3/2) linked by corner-sharing in the ab-plane. The M spins interact with each other via four different antiferromagnetic exchange interactions, J1, J2, J3 and J4. Despite the considerable geometrical frustration, Li3Mg2MO6 exhibits an antiferromagnetic long-range order at TN = 18 K for M = Ru and TN = 8 K for M = Os. Heat capacity...
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