uSR study of low temperature magnetism in Li NMC 811

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LiNi0.8Mn0.1Co0.1O2 (Li NMC 811) is a next generation Li ion battery cathode material. We are investigating the magnetic properties of Li NMC 811 to track the changes in local ordering of the magnetic ions and changes in oxidation state as a function of electrochemical cycling. Here we focus on pristine Li NMC 811 which contains S=1/2 Ni3+, S=1 Ni2+, S=3/2 Mn4+ and S=0 Co3+. In addition it is prone to off-stoichiometry and Li/Ni site disorder...
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