Hydration behaviour of uranyl chloride: from fundamental chemistry to environmental applications

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In water uranium exists almost exclusively as the uranyl ion [UO2]2+. In the presence of halides these can form complexes of the type [UO2(H2O)nClx]2-x, whose thermodynamics and structures in solution are not fully understood. This is important as high halide concentrations are expected to be found in spent nuclear fuels or under certain environmental conditions. In this work we propose to study the reaction of uranyl chloride [UO2(H2O)5][Cl]2 with LiCl under increasing halide concentrations to...
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