BoxCARS 2D IR Spectroscopy with Pulse Shaping

Ziareena Al-Mualem, Xiaobing Chen, Joseph Shirley, Cong Xu & Carlos Baiz
BoxCARS and pump-probe geometries are common implementations of two dimensional infrared (2D IR) spectroscopy. BoxCARS is background-free, generally offering greater signal to noise ratio, which enables measuring weak vibrational echo signals. Pulse shapers have been implemented in the pump probe geometry to accelerate data collection and suppress scatter and other unwanted signals by precise control of the pump pulse delay and carrier phase. Here, we introduce a 2D IR optical setup in the BoxCARS geometry...
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