Nonlinear phase-modulated spectroscopy of doped helium droplet beams and dilute gases

Lukas Bruder
This dissertation focuses on the application of nonlinear time-domain spectroscopy to cold helium nanodroplet beams and dilute atomic vapors. Femtosecond pump-probe wave packet interferometry is performed to track the coherent evolution of electronic and vibronic wave packets induced in the systems. To this end, a phase modulation technique is implemented to enhance the sensitivity and resolution in the experiments. Rubidium atoms attached to helium droplets are investigated as well as rubidium-helium excimers that form on...
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